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Decommissioning & Environmental Sciences
The mission of the Decommissioning and Environmental Sciences (DES) Division is to promote the development and use of those skills and technologies associated with the use of nuclear energy and the optimal management and stewardship of the environment, sustainable development, decommissioning, remediation, reutilization, and long-term surveillance and maintenance of nuclear-related installations, and sites. The target audience for this effort is the membership of the Division, the Society, and the public at large.
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Latest News
First astatine-labeled compound shipped in the U.S.
The Department of Energy’s National Isotope Development Center (NIDC) on March 31 announced the successful long-distance shipment in the United States of a biologically active compound labeled with the medical radioisotope astatine-211 (At-211). Because previous shipments have included only the “bare” isotope, the NIDC has described the development as “unleashing medical innovation.”
Anatoly Bushuev, Alexander Kozhin, Viktor Zubarev, Tatiana Aleeva, Ekaterina Petrova, Anatoly Myrzin, Alexey Syrosev, Genadiy Vlaskin, Timur Ragimov, Valentin Timoshin, Andrey Samoilov
Nuclear Technology | Volume 170 | Number 2 | May 2010 | Pages 353-359
Technical Paper | Human Factors | doi.org/10.13182/NT10-A9488
Articles are hosted by Taylor and Francis Online.
This paper presents a nondestructive methodology for the determination of mass and isotopic composition of large plutonium samples. The methodology is based on experimental data from measurements of gamma radiation emitted by plutonium samples under assay. Both plutonium mass and plutonium isotopic composition are derived from one experimental gamma spectrum in two energy ranges. Gamma spectrum in the middle-energy range is used for the determination of plutonium isotopic composition from experimental intensities of photo peaks belonging to different plutonium isotopes. Gamma spectrum in the high-energy range contains photo peaks of spontaneous fission products, and these data can be used for the determination of plutonium mass. The calibration curve for dependence of the count rates in photo peaks of spontaneous fission products on effective 240Pu mass was plotted based on experimental data for the enterprise-level reference plutonium samples. When processing experimental data, some corrections were introduced to account for self-absorption of gamma radiation in the plutonium samples and for neutron-induced fission reactions. The correction factors were calculated with the application of Monte Carlo methodology. The final relative errors in the determination of plutonium dioxide mass were within the range of (4 to 10)% (1) for nuclear material containers with different cooling times and different isotopic compositions of plutonium.
