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April 3–5, 2025
Albuquerque, NM|The University of New Mexico
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Latest News
First astatine-labeled compound shipped in the U.S.
The Department of Energy’s National Isotope Development Center (NIDC) on March 31 announced the successful long-distance shipment in the United States of a biologically active compound labeled with the medical radioisotope astatine-211 (At-211). Because previous shipments have included only the “bare” isotope, the NIDC has described the development as “unleashing medical innovation.”
Mélany Gouëllo, Jouni Hokkinen, Teemu Kärkelä, Ari Auvinen
Nuclear Technology | Volume 203 | Number 1 | July 2018 | Pages 66-84
Technical Paper | doi.org/10.1080/00295450.2018.1429111
Articles are hosted by Taylor and Francis Online.
This work is a contribution toward understanding the chemical reactions on the primary circuit surfaces involving gaseous iodine release during a severe nuclear reactor accident. Cesium iodide was used as a nonradioactive precursor material in order to highlight the effects of carrier gas composition (Ar/H2O, Ar/H2O/H2, and Ar/Air), temperature, the initial cesium/iodine (Cs/I) molar ratio by adding cesium hydroxide, and the presence of boron on the molar composition of the deposited iodine compound and on the release of gaseous iodine from the deposit. The results from the experiments involving only cesium iodide as a precursor revealed a slight decomposition of cesium iodide and a release of gaseous iodine. Furthermore, the measured gaseous iodine mass decreased with the addition of hydrogen to the carrier gas at 650°C. At 400°C, the amount of released material (aerosol and gas) was decreased. However, whereas at 650°C the sampled iodine existed mainly as aerosols, the mass concentration recorded from the experiment at 400°C indicated a predominance of gaseous iodine. When the initial Cs/I molar ratio was significantly greater than unity (1.5 < Cs/I < 4.5), the mass of produced gaseous iodine was barely detectable, suggesting a reaction between cesium hydroxide and the gaseous iodine released from cesium iodide decomposition. In the presence of boron, the transport of gaseous iodine was increased as a result of the formation of glassy cesium borate in the evaporation crucible. The presence of steam and its quantity were shown to have an enhancing influence on the cesium borate formation and on the release of gaseous iodine.