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April 3–5, 2025
Albuquerque, NM|The University of New Mexico
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Latest News
First astatine-labeled compound shipped in the U.S.
The Department of Energy’s National Isotope Development Center (NIDC) on March 31 announced the successful long-distance shipment in the United States of a biologically active compound labeled with the medical radioisotope astatine-211 (At-211). Because previous shipments have included only the “bare” isotope, the NIDC has described the development as “unleashing medical innovation.”
Hilbert Christensen
Nuclear Technology | Volume 155 | Number 3 | September 2006 | Pages 358-364
Technical Paper | Materials for Nuclear Systems | doi.org/10.13182/NT06-A3768
Articles are hosted by Taylor and Francis Online.
A previously developed radiolysis model has been used to simulate experiments from four laboratories. The source strengths in the experiments with UO2, doped with 238Pu, were 0.01, 0.1, and 1 Ci/g. The agreement was good with the experimental results of Stroes-Gascoyne et al. for their sample with 0.1 Ci/g. Their sample containing 0.01 Ci/g gave a factor-of-3-higher calculated corrosion rate compared with the experimental rate. In the experiments of Cobos et al. and of Kelm and Bohnert, using alpha-doped UO2, the calculated corrosion rates were somewhat lower than the experimental rates. However, recent experiments by Rondinella et al. using UO2 with 10% doped 233U gave considerably lower corrosion rates in good agreement with the model. The calculated corrosion rates for the same source strength were about the same for the experiments by Stroes-Gascoyne et al., Kelm and Bohnert, and Cobos et al. However, the experimental rates varied considerably. The agreement was not good with experiments using Pu(VI) dissolved in solution, in which case the calculated corrosion rate was ten times or more than ten times lower than the experimental rate. The reason for this disagreement could be a chemical effect of Pu(VI) in the solution.