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General Kenneth Nichols and the Manhattan Project
Nichols
The Oak Ridger has published the latest in a series of articles about General Kenneth D. Nichols, the Manhattan Project, and the 1954 Atomic Energy Act. The series has been produced by Nichols’ grandniece Barbara Rogers Scollin and Oak Ridge (Tenn.) city historian David Ray Smith. Gen. Nichols (1907–2000) was the district engineer for the Manhattan Engineer District during the Manhattan Project.
As Smith and Scollin explain, Nichols “had supervision of the research and development connected with, and the design, construction, and operation of, all plants required to produce plutonium-239 and uranium-235, including the construction of the towns of Oak Ridge, Tennessee, and Richland, Washington. The responsibility of his position was massive as he oversaw a workforce of both military and civilian personnel of approximately 125,000; his Oak Ridge office became the center of the wartime atomic energy’s activities.”
M. Gonzalez, L. Hansen, D. Rappleye, R. Cumberland, M. F. Simpson
Nuclear Technology | Volume 192 | Number 2 | November 2015 | Pages 165-171
Technical Paper | Reprocessing | doi.org/10.13182/NT15-28
Articles are hosted by Taylor and Francis Online.
It has previously been proposed by safeguards experts that curium will track plutonium through a spent fuel pyroprocessing facility, enabling nondestructive assaying of plutonium via counting neutron emissions from 244Cm. This is a critical assumption for the neutron balance approach to safeguards. If Cm and Pu were to behave chemically the same, counting neutrons could be used to estimate Pu concentrations. In this study, plutonium tracking with curium has been investigated using Enhanced REFIN with Anodic Dissolution (ERAD), a one-dimensional transient electrorefiner model based on fundamental electrochemical equations. The model was used to simulate simultaneous deposition of uranium, plutonium, and curium onto a solid metal cathode. Chemical/physical properties used by the model were either obtained from the literature or assumed. The standard exchange current density of curium was estimated by analyzing published cyclic voltammetry data for LiCl-KCl-CmCl3. The focus of the ERAD calculations was on verifying that Pu and Cm could codeposit onto the cathode along with U and to determine if the Pu/Cm ratio would be the same between the salt pool and cathode deposit. It was determined that Cm largely resists cathode deposition, while Pu can be driven to codeposit at sufficiently high current densities. The expected concentration of Cm in the salt would not support any deposition of Cm onto the cathode. It would need to be raised to ~1 wt% before small gram quantities of Cm will deposit onto the cathode. Even then, the Pu/Cm ratio of the cathode was found to be three orders of magnitude higher than the ratio in the salt. It is, thus, concluded that the neutron balance approach would be ineffective at safeguarding a nuclear fuel pyroprocessing facility.