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First astatine-labeled compound shipped in the U.S.
The Department of Energy’s National Isotope Development Center (NIDC) on March 31 announced the successful long-distance shipment in the United States of a biologically active compound labeled with the medical radioisotope astatine-211 (At-211). Because previous shipments have included only the “bare” isotope, the NIDC has described the development as “unleashing medical innovation.”
Bassam I. Shamoun, Robert J. Witt
Nuclear Technology | Volume 107 | Number 2 | August 1994 | Pages 227-235
Technical Note | Nuclear Reactor Safety | doi.org/10.13182/NT94-A34989
Articles are hosted by Taylor and Francis Online.
Recriticality is possible in a severe accident if unborated or low boron concentration water is added to a damaged core after control rod melting but before fuel melting. Recriticality in a severe accident in a boiling water reactor was parametrically investigated using the TWODANT code. Eigenvalue calculations for a unit central fuel cell with reflective boundary conditions were performed by solving the two-dimensional multigroup steady-state Boltzman transport equation using TWODANT. Two sets of calculations were performed in this work. The first set of calculations was carried out under three types of normal operating conditions to provide reference values for the accident calculations: (a) cold rodded condition, (b) cold unrodded condition, and (c) hot full-power condition. The eigenvalues at these conditions were found to be 1.055, 1.208, and 1.098, respectively. The second set of calculations was carried out after the melting of the control element and during the reflood phase, under the following reflood conditions: (a) reflood with unborated water and (b) reflood with borated water. For the reflood case with unborated water, five values of void fractions were considered (100, 60, 40, 20, and 0%). Decreasing void fractions represent greater refill levels during the reflood process. The system pressure was taken to be 7 MPa, while the moderator temperature was set to 560 K. Plotting the eigenvalue compared with the fraction of control materials lost indicates recriticality is only possible if nearly 100% of the control material is lost from the core. Eigenvalue calculations were repeated for short- and long-term recovery conditions of the reflood phase corresponding to maximum moderator density at 4 MPa pressure and 525 K moderator temperature and for 1 MPa pressure and 325 K moderator temperature, respectively. Recriticality was again observed to be a concern only after losing 95% or more of control materials from the unit cell. Although a three-dimensional treatment might not require such a large percentage loss, these results suggest recriticality is not a major issue as there is likely to be significant fuel slumping before 95 % of the control material leaves the core.