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Isotopes & Radiation
Members are devoted to applying nuclear science and engineering technologies involving isotopes, radiation applications, and associated equipment in scientific research, development, and industrial processes. Their interests lie primarily in education, industrial uses, biology, medicine, and health physics. Division committees include Analytical Applications of Isotopes and Radiation, Biology and Medicine, Radiation Applications, Radiation Sources and Detection, and Thermal Power Sources.
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2024 ANS Winter Conference and Expo
November 17–21, 2024
Orlando, FL|Renaissance Orlando at SeaWorld
Standards Program
The Standards Committee is responsible for the development and maintenance of voluntary consensus standards that address the design, analysis, and operation of components, systems, and facilities related to the application of nuclear science and technology. Find out What’s New, check out the Standards Store, or Get Involved today!
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Latest News
Siting of Canadian repository gets support of tribal nation
Canada’s Nuclear Waste Management Organization (NWMO) announced that Wabigoon Lake Ojibway Nation has indicated its willingness to support moving forward to the next phase of the site selection process to host a deep geological repository for Canada’s spent nuclear fuel.
Masatoshi Iizuka, Masaaki Akagi, Takashi Omori
Nuclear Technology | Volume 181 | Number 3 | March 2013 | Pages 507-525
Technical Papers | Reprocessing | doi.org/10.13182/NT13-A15807
Articles are hosted by Taylor and Francis Online.
A new treatment process was proposed for the anode residue from a molten salt electrorefining step in the pyrometallurgical reprocessing of spent metallic fast reactor fuel. This treatment process consists of two steps: (a) oxidation of the remaining actinides in the anode residue by the addition of CdCl2 and (b) removal of the accompanying chloride by high-temperature distillation. The oxidation of the remaining uranium by CdCl2 was studied using anode residue from previous electrorefining experiments using U-Zr alloys. The reaction between uranium and CdCl2 was completed in [approximately]2 days with a satisfactory chlorine balance among the species in the molten chlorides solvent. A high uranium oxidation rate was attained by appropriately controlling the rate of CdCl2 addition. The high-temperature distillation tests were carried out at 1473 K with pressure of [approximately]300 Pa to remove the solvent accompanying the anode residue. The chloride content in the anode residue was lowered to 1% to 2.5% by the distillation operation. Although the anode residue was heated to 1673 to 1773 K at a pressure of [approximately]50 kPa after the distillation, it was not melted completely. The remaining ratio of uranium after the electrorefining and the above treatment process was evaluated to be 0.04% to 0.20%. Material flow calculations were performed for a pyrometallurgical reprocessing facility equipped with the anode residue treatment process. It showed that (a) the chlorine and uranium supply/demand balance is maintained unless the remaining ratio of uranium after electrorefining exceeds a certain value and (b) the addition of the anode residue treatment process does not have an adverse effect on either the performance of the overall process or the facility design.