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General Kenneth Nichols and the Manhattan Project
Nichols
The Oak Ridger has published the latest in a series of articles about General Kenneth D. Nichols, the Manhattan Project, and the 1954 Atomic Energy Act. The series has been produced by Nichols’ grandniece Barbara Rogers Scollin and Oak Ridge (Tenn.) city historian David Ray Smith. Gen. Nichols (1907–2000) was the district engineer for the Manhattan Engineer District during the Manhattan Project.
As Smith and Scollin explain, Nichols “had supervision of the research and development connected with, and the design, construction, and operation of, all plants required to produce plutonium-239 and uranium-235, including the construction of the towns of Oak Ridge, Tennessee, and Richland, Washington. The responsibility of his position was massive as he oversaw a workforce of both military and civilian personnel of approximately 125,000; his Oak Ridge office became the center of the wartime atomic energy’s activities.”
Masatoshi Iizuka, Masaaki Akagi, Takashi Omori
Nuclear Technology | Volume 181 | Number 3 | March 2013 | Pages 507-525
Technical Papers | Reprocessing | doi.org/10.13182/NT13-A15807
Articles are hosted by Taylor and Francis Online.
A new treatment process was proposed for the anode residue from a molten salt electrorefining step in the pyrometallurgical reprocessing of spent metallic fast reactor fuel. This treatment process consists of two steps: (a) oxidation of the remaining actinides in the anode residue by the addition of CdCl2 and (b) removal of the accompanying chloride by high-temperature distillation. The oxidation of the remaining uranium by CdCl2 was studied using anode residue from previous electrorefining experiments using U-Zr alloys. The reaction between uranium and CdCl2 was completed in [approximately]2 days with a satisfactory chlorine balance among the species in the molten chlorides solvent. A high uranium oxidation rate was attained by appropriately controlling the rate of CdCl2 addition. The high-temperature distillation tests were carried out at 1473 K with pressure of [approximately]300 Pa to remove the solvent accompanying the anode residue. The chloride content in the anode residue was lowered to 1% to 2.5% by the distillation operation. Although the anode residue was heated to 1673 to 1773 K at a pressure of [approximately]50 kPa after the distillation, it was not melted completely. The remaining ratio of uranium after the electrorefining and the above treatment process was evaluated to be 0.04% to 0.20%. Material flow calculations were performed for a pyrometallurgical reprocessing facility equipped with the anode residue treatment process. It showed that (a) the chlorine and uranium supply/demand balance is maintained unless the remaining ratio of uranium after electrorefining exceeds a certain value and (b) the addition of the anode residue treatment process does not have an adverse effect on either the performance of the overall process or the facility design.