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ANS Student Conference 2025
April 3–5, 2025
Albuquerque, NM|The University of New Mexico
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General Kenneth Nichols and the Manhattan Project
Nichols
The Oak Ridger has published the latest in a series of articles about General Kenneth D. Nichols, the Manhattan Project, and the 1954 Atomic Energy Act. The series has been produced by Nichols’ grandniece Barbara Rogers Scollin and Oak Ridge (Tenn.) city historian David Ray Smith. Gen. Nichols (1907–2000) was the district engineer for the Manhattan Engineer District during the Manhattan Project.
As Smith and Scollin explain, Nichols “had supervision of the research and development connected with, and the design, construction, and operation of, all plants required to produce plutonium-239 and uranium-235, including the construction of the towns of Oak Ridge, Tennessee, and Richland, Washington. The responsibility of his position was massive as he oversaw a workforce of both military and civilian personnel of approximately 125,000; his Oak Ridge office became the center of the wartime atomic energy’s activities.”
Byung-Gil Ahn, Hwan-Seo Park, In-Tae Kim, Han-Soo Lee
Nuclear Technology | Volume 173 | Number 3 | March 2011 | Pages 300-309
Technical Paper | Radioactive Waste Management and Disposal | doi.org/10.13182/NT11-A11663
Articles are hosted by Taylor and Francis Online.
The waste generated from a pyrochemical process to recover uranium and transuranic elements has been one of the problematic wastes because of high volatility and low compatibility with silicate glass. For the minimization of final waste, an oxidative precipitation by sparging oxygen has been under development, and the waste containing rare earth oxides (REOs) and volatile salt is expected to be generated. This study intended to find a way to immobilize these kinds of wastes under the limitations of a processing temperature ([approximately]1200°C) and a waste loading ([approximately]20 wt%). From a series of consolidation experiments, it was induced that Ca-rich silicate glass is effective in consolidating the REOs at relatively low temperature. Based on this result, CaO-SiO2-P2O5 (CaPS) was designed to provide a way to control the volatility of waste and to avoid glass effects in the consolidation at a given temperature. By using a CaPS, REOs were consolidated, regardless of glass composition. At a high content of metal chlorides, CaPS can control the volatility up to 1200°C, but it has a low ability to immobilize alkali metal elements. For this, SiO2-Al2O3-P2O5 (SAP) was suggested to treat LiCl-KCl salt in precipitate. This composite can also control the volatility up to 1200°C, and it converted the REOs into monazite at 650°C, where the entire metal elements in chloride form are changed into relatively stable compounds. The leach test by the product consistency test-method A confirmed the immobilization ability of SAP for waste with a high content of metal chlorides. In conclusion, this study suggests the approach concept to treat a waste containing volatile compounds. For a lower content of metal chloride, CaPS are more favorable, and for a high content of metal chlorides, SAP is more effective to fabricate a wasteform for final disposal.