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IAEA project aims to develop polymer irradiation model
The International Atomic Energy Agency has launched a new coordinated research project (CRP) aimed at creating a database of polymer-radiation interactions in the next five years with the long-term goal of using the database to enable machine learning–based predictive models.
Radiation-induced modifications are widely applicable across a range of fields including healthcare, agriculture, and environmental applications, and exposure to radiation is a major factor when considering materials used at nuclear power plants.
Lance Davis, Ralph Hania, Dennis Boomstra, Dillon Rossouw, Florence Charpin-Jacobs, Jan Uhlir, Martin Maracek, Helmut Beckers, Sebastian Riedel
Nuclear Science and Engineering | Volume 197 | Number 4 | April 2023 | Pages 633-646
Technical Paper | doi.org/10.1080/00295639.2022.2129951
Articles are hosted by Taylor and Francis Online.
Radiolytic fluorine gas production at temperatures of 40°C to 60°C was investigated for the fluoride salts LiF, BeF2, UF4, ThF4, and 71.7LiF-16BeF2-12.3UF4 (FliBe-UF4) by gamma irradiation of powdered samples using spent fuel elements from the High Flux Reactor (HFR) Petten as the irradiation source; work of a similar nature was previously performed at Oak Ridge National Laboratory in the period 1965 to 1995. Gamma irradiation was conducted for just over 41 days, with total absorbed gamma dose ranging from ~45 MGy for the lightest salts to ~170 MGy for ThF4 and UF4. By measuring the gas pressure within salt-filled capsules during irradiation, it was possible to quantify radiolytic gas production for all salt samples except UF4. Production rates are reported as the salt G-values, measured as number of fluorine molecules produced per 100 eV of energy absorbed (molecules F2/100 eV). The G-values of the salts were found to be G(LiF) ~0.004, G(BeF2) ~0.009, G(ThF4) ~0.021, and G(FLiBe-UF4) ~0.005.
