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60 Years of U: Perspectives on resources, demand, and the evolving role of nuclear energy
Recent years have seen growing global interest in nuclear energy and rising confidence in the sector. For the first time since the early 2000s, there is renewed optimism about the industry’s future. This change is driven by several major factors: geopolitical developments that highlight the need for secure energy supplies, a stronger focus on resilient energy systems, national commitments to decarbonization, and rising demand for clean and reliable electricity.
T. A. Gens, R. E. Blanco
Nuclear Science and Engineering | Volume 11 | Number 3 | November 1961 | Pages 267-273
Technical Paper | doi.org/10.13182/NSE61-A26002
Articles are hosted by Taylor and Francis Online.
A Modified Zirflex process was developed in the laboratory for dissolution of 1–10 % uranium-zirconium alloy fuels clad in Zircaloy-2 to produce a nitrate solution from which uranium can be recovered by conventional solvent extraction methods. A flowsheet is presented for dissolution of 7% uranium-zirconium alloy in 5.4 M NH4F-0.33 M NH4NO3. Enough 1 M H2O2 is added continually during dissolution to yield 0.13 M H2O2 in the final solution, neglecting the amount reacting. Dissolution of a 70-mil thick sample is complete in 1 hr. The solvent extraction feed is prepared by adding aluminum nitrate and nitric acid to the dissolver solution to yield a stable solvent extraction feed solution of 0.0075 M uranium, 0.25 M zirconium, 1 M aluminum, 2 M fluoride, and 1 M nitric acid. The off-gas is approximately 98.5% NH6, 1% H2, 0.3% O2, and 0.2% N2. Conventional stainless steel such as 309SNb or Hastelloy F appear to be suitable materials of construction with corrosion rates varying from 0.1 to 3.0 mils/month.
