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ANS Student Conference 2025
April 3–5, 2025
Albuquerque, NM|The University of New Mexico
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First astatine-labeled compound shipped in the U.S.
The Department of Energy’s National Isotope Development Center (NIDC) on March 31 announced the successful long-distance shipment in the United States of a biologically active compound labeled with the medical radioisotope astatine-211 (At-211). Because previous shipments have included only the “bare” isotope, the NIDC has described the development as “unleashing medical innovation.”
T. J. van Rooyen, G. P. de Beer
Nuclear Science and Engineering | Volume 114 | Number 2 | June 1993 | Pages 87-101
Technical Paper | doi.org/10.13182/NSE93-A24020
Articles are hosted by Taylor and Francis Online.
Prompt fission neutrons (PFNs) constitute the most important component of the source term for nuclear reactor shielding calculations. The determination of the PFN source term for reactor shielding calculations has traditionally been performed using a number of simplifying assumptions. Very simple closed analytical expressions are normally used for the PFN spectrum. The Watt PFN spectrum for 235U, with coefficients determined by Cranberg et al., has become a virtual industry standard in the reactor shielding community. The source term is usually treated as a separable function of spatial location and energy, only the 235U spectrum is considered, and the effect of burnup on the source term is neglected. In reality, the PFN spectra of 235U, 238U, and 239Pu differ markedly, and their fractional contributions to fission are a function of burnup, which, in turn, is a time-dependent function of the spatial position within the reactor core. Recent theoretical developments have led to the advent of sophisticated microscopic models for the calculation of PFN spectra and multiplicities of various fissioning systems. Spectra for 235U, 238U, and 239Pu, calculated with the Madland-Nix model with fragment spin correction, were used in this investigation. An improved reactor source term model that calculates spectrally and spatially burnup-compensated source terms for nuclear reactor shielding calculations is developed and applied to a typical light water reactor (LWR).,Neutron, gamma-ray, and total absorbed dose rate distributions were calculated through four diverse biological shields with a thickness of 250 cm. At end-of-life core conditions, the traditional source term model leads to an underestimate of the transmitted absorbed dose rates by slightly more than a factor of 2. This discrepancy lies within the error margins quoted for LWR shielding calculations. We conclude that despite their age and simplicity, the Watt formula and the simple source term model are of sufficient accuracy for continued service. The more rigorous source term model presented here may be useful for accurate benchmark calculations and for the design of highly efficient shields for high-burnup reactors.