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Members are devoted to applying nuclear science and engineering technologies involving isotopes, radiation applications, and associated equipment in scientific research, development, and industrial processes. Their interests lie primarily in education, industrial uses, biology, medicine, and health physics. Division committees include Analytical Applications of Isotopes and Radiation, Biology and Medicine, Radiation Applications, Radiation Sources and Detection, and Thermal Power Sources.
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General Kenneth Nichols and the Manhattan Project
Nichols
The Oak Ridger has published the latest in a series of articles about General Kenneth D. Nichols, the Manhattan Project, and the 1954 Atomic Energy Act. The series has been produced by Nichols’ grandniece Barbara Rogers Scollin and Oak Ridge (Tenn.) city historian David Ray Smith. Gen. Nichols (1907–2000) was the district engineer for the Manhattan Engineer District during the Manhattan Project.
As Smith and Scollin explain, Nichols “had supervision of the research and development connected with, and the design, construction, and operation of, all plants required to produce plutonium-239 and uranium-235, including the construction of the towns of Oak Ridge, Tennessee, and Richland, Washington. The responsibility of his position was massive as he oversaw a workforce of both military and civilian personnel of approximately 125,000; his Oak Ridge office became the center of the wartime atomic energy’s activities.”
Vojtěch Galek, Anna Sears, Petr Pražák, Lucie Karásková-Nenadálová
Fusion Science and Technology | Volume 80 | Number 3 | May 2024 | Pages 321-329
Research Article | doi.org/10.1080/15361055.2024.2305996
Articles are hosted by Taylor and Francis Online.
Tritium is a radioactive isotope of hydrogen, and due to its limited supply and related high price, it is necessary to recover it from tritiated materials via detritiation technologies. The number of tritiated materials arises during fusion. Tritium from fusion reactors is deposited in the outer layer of plasma-facing materials, which must be dealt with during maintenance or decommissioning processes. A second source of waste is laboratory equipment that could be contaminated with tritium.
High-temperature treatment in an oxidation environment can achieve the release of tritium from metals or organic materials. The tritiated vapor is then captured in a series of water bubblers and reprocessed into pure T2. One of the high-temperature methods is molten salt oxidation (MSO), which uses high temperatures, alkaline salt, and an oxidative environment for flameless oxidation of different types of waste.
This work aimed to simulate the detritiation processes of tritiated organic materials in MSO technology. First, a series of experiments with D2O absorbed in ion resins was conducted. The organic waste was decomposed within the molten salt, and the flue gas was measured to determine the oxidation efficiency. The D2O was captured in a series of water bubblers, and the water was then analyzed with attenuated total reflectance (ATR)–Fourier transform infrared spectroscopy (FTIR). The results showed that all deuterium in the form of D2O was caught in the first water bubbler. The capture efficiency ranged from 22.32% to 61.13%. The lower efficiency capture can be explained as D2O in water can form a HDO molecule and its correct determination is problematic.
The second type of experiment was carried out with T2O with an activity of 851 Bq and with tritiated oil with an activity of 2495 Bq. The T2O was added to the set amount of ion resins and dosed into MSO. A peristaltic pump dosed the tritiated oil. The flue gas was measured to determine oxidation efficiency, and the T2O was captured within the water bubblers. The water was analyzed with liquid scintillation spectroscopy. The capture efficiency ranged between 76.42% to 97.87%. The results showed that this technology is suitable for the detritiation of tritiated organic materials.
