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Fusion Science and Technology
Latest News
Argonne research aims to improve nuclear fuel recycling and metal recovery
Servis
Scientists at Argonne National Laboratory are investigating a used nuclear fuel recycling technology that could lead to a scaled-down and more efficient approach to metal recovery, according to a recent news article from the lab. The research, led by Argonne radiochemist Anna Servis with funding from the Department of Energy’s Advanced Research Projects Agency–Energy (ARPA-E), could have an impact beyond the nuclear fuel cycle and improve other high-value metal processing, such as rare earth recovery, according to Argonne.
The research: Servis’s work is being carried out under ARPA-E’s CURIE (Converting UNF Radioisotopes Into Energy) program. The specific project—Radioisotope Capture Intensification Using Rotating Packed Bed Contactors—started in 2023 and is scheduled to end in January 2026.
Y. E. Titarenko, S. S. Ananev, V. F. Batyaev, V. I. Belousov, V. Y. Blandinskiy, K. G. Chernov, V. D. Davidenko, A. A. Dudnikov, I. I. Dyachkov, M. V. Ioannisian, A. A. Kovalishin, V. I. Khripunov, B. V. Kuteev, V. O. Legostaev, M. R. Malkov, K. V. Pavlov, A. Y. Titarenko, M. A. Zhigulina, V. M. Zhivun, Y. A. Kashchuk, S. A. Meshchaninov, S. Y. Obudovsky, A. Y. Stankovskiy, A. Y. Konobeyev
Fusion Science and Technology | Volume 79 | Number 2 | February 2023 | Pages 117-134
Technical Paper | doi.org/10.1080/15361055.2022.2121525
Articles are hosted by Taylor and Francis Online.
This paper presents the results of the experimental determination and computational simulation of the ambient dose equivalent rate for a metallic thorium cylindrical miniblock and the (n,2n), (n,f), and (n,γ) reaction rates in a thin 232Th metal foil irradiated with neutrons of the NG-24M generator spectrum. The ambient dose equivalent rate was determined by dosimeters-radiometers. The reaction rates were determined by the activation method using Ge spectrometers without destroying the irradiated samples. Computational simulations of ambient dose equivalent and reaction rates were performed, respectively, using the radiation transport codes PHITS, MCNP5, and KIR2, which use various nuclear data libraries: JEFF-3.2 and -3.3; JENDL4.0; ENDF/B-VII.0, -VII.1, and -VIII.0; ROSFOND; FENDL; and TENDL. The authors give an estimate of the 232U/233U relative accumulation upon natural thorium irradiation in a fusion facility blanket with defined neutron spectrum. The nonirradiated and irradiated thorium nuclide composition change simulation and visualization were performed using analytical solutions of an ordinary system of homogeneous linear differential equations describing nuclide transmutations.