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Fusion Science and Technology
Latest News
Argonne research aims to improve nuclear fuel recycling and metal recovery
Servis
Scientists at Argonne National Laboratory are investigating a used nuclear fuel recycling technology that could lead to a scaled-down and more efficient approach to metal recovery, according to a recent news article from the lab. The research, led by Argonne radiochemist Anna Servis with funding from the Department of Energy’s Advanced Research Projects Agency–Energy (ARPA-E), could have an impact beyond the nuclear fuel cycle and improve other high-value metal processing, such as rare earth recovery, according to Argonne.
The research: Servis’s work is being carried out under ARPA-E’s CURIE (Converting UNF Radioisotopes Into Energy) program. The specific project—Radioisotope Capture Intensification Using Rotating Packed Bed Contactors—started in 2023 and is scheduled to end in January 2026.
Bogdan Florian Monea, Eusebiu Ilarian Ionete, Catalin Ducu, Stefan Ionut Spiridon, Sorin Moga, Xingbo Han, Wei Liu
Fusion Science and Technology | Volume 77 | Number 5 | July 2021 | Pages 382-390
Technical Paper | doi.org/10.1080/15361055.2021.1903782
Articles are hosted by Taylor and Francis Online.
In the present study, the effect of Hf and Ti substitution of Zr in the ZrCo alloy, used for hydrogen isotope storage, has been investigated in order to ascertain the improvement of the anti-disproportionation property of ZrCo hydrides. The ultimate goal of the investigation is to develop a safe and economically viable solution for the long-term storage of deuterium and tritium. The intermetallic compounds Zrl-xTixCo and Zrl-xHfxCo (x = 0.1, 0.2) were prepared and their suitability for hydrogen isotope storage, protium (H) and deuterium (D), was investigated. The alloys were synthesized by arc melting under a controlled argon atmosphere and characterized by scanning electron microscope and X-ray diffraction analysis. The hydrogen isotope storage behavior of these alloys was probed by loading and unloading protium and deuterium. We present the pressure, composition, and temperature measurements for desorption, together with the thermodynamic parameters (enthalpy and entropy) of these alloys. The experimental results show that Ti and Hf substitution in the ZrCo alloys is suitable for fast delivery of hydrogen isotopes, even after their long-term storage.
