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Argonne research aims to improve nuclear fuel recycling and metal recovery
Servis
Scientists at Argonne National Laboratory are investigating a used nuclear fuel recycling technology that could lead to a scaled-down and more efficient approach to metal recovery, according to a recent news article from the lab. The research, led by Argonne radiochemist Anna Servis with funding from the Department of Energy’s Advanced Research Projects Agency–Energy (ARPA-E), could have an impact beyond the nuclear fuel cycle and improve other high-value metal processing, such as rare earth recovery, according to Argonne.
The research: Servis’s work is being carried out under ARPA-E’s CURIE (Converting UNF Radioisotopes Into Energy) program. The specific project—Radioisotope Capture Intensification Using Rotating Packed Bed Contactors—started in 2023 and is scheduled to end in January 2026.
Shouxi Gu, Qiang Qi, Yingchun Zhang, Baolong Ji, Haishan Zhou, Guang-Nan Luo
Fusion Science and Technology | Volume 76 | Number 4 | May 2020 | Pages 536-542
Technical Paper | doi.org/10.1080/15361055.2020.1718950
Articles are hosted by Taylor and Francis Online.
Core-shell Li2TiO3-Li4SiO4 has been suggested as an advanced tritium breeder for outstanding mechanical strength and rich lithium. However, no study has reported on the release behavior of hydrogen isotopes from core-shell Li2TiO3-Li4SiO4. This paper focuses on a deuterium exposure experiment to investigate deuterium release behavior. X-ray diffraction, Raman, and electron spin resonance measurements were adopted to analyze the phase change, crystal structure modification, and defects before and after deuterium exposure. Thermal desorption spectroscopy was used to study the deuterium release behavior of core-shell Li2TiO3-Li4SiO4. Deuterium release from single Li4SiO4 and Li2TiO3 was also examined for comparison. The similarity of the deuterium release profiles between core-shell Li2TiO3-Li4SiO4 and Li4SiO4 was observed, which was considered to be caused by the incomplete coverage of shell Li2TiO3 on the core-shell samples.