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Argonne research aims to improve nuclear fuel recycling and metal recovery
Servis
Scientists at Argonne National Laboratory are investigating a used nuclear fuel recycling technology that could lead to a scaled-down and more efficient approach to metal recovery, according to a recent news article from the lab. The research, led by Argonne radiochemist Anna Servis with funding from the Department of Energy’s Advanced Research Projects Agency–Energy (ARPA-E), could have an impact beyond the nuclear fuel cycle and improve other high-value metal processing, such as rare earth recovery, according to Argonne.
The research: Servis’s work is being carried out under ARPA-E’s CURIE (Converting UNF Radioisotopes Into Energy) program. The specific project—Radioisotope Capture Intensification Using Rotating Packed Bed Contactors—started in 2023 and is scheduled to end in January 2026.
Asset Shaimerdenov, Shamil Gizatulin, Daulet Dyussambayev, Saulet Askerbekov, Inesh Kenzhina
Fusion Science and Technology | Volume 76 | Number 3 | April 2020 | Pages 304-313
Technical Paper | doi.org/10.1080/15361055.2020.1711852
Articles are hosted by Taylor and Francis Online.
The WWR-K is 6-MW(thermal) light-water, tank-type reactor with thermal neutron spectrum. It is the exclusive multipurpose research reactor in the Republic of Kazakhstan. The WWR-K is owned by the Institute of Nuclear Physics of the Ministry of Energy of the Republic of Kazakhstan. The coolant is desalted water. The moderator and the reflector are desalted water and beryllium. The reactor operates on uranium dioxide that is enriched to 19.7% by 235U. The reactor is equipped with irradiation channels with the following characteristics: the thermal neutron flux density in the core center comprises 2 · 1014 cm−2s−1, whereas the fast neutron flux density (En > 0.1 MeV) comprises ~8 · 1013 cm−2s−1; in the core periphery, fluxes of the thermal and fast neutrons comprise, respectively, ~8 · 1013 and ~6 · 1012 cm−2s−1. The regular irradiation cycle length is 21 days. The annual number of cycles is ten.
Since WWR-K reactor startup, the studies of various prospective reactor materials and fuels have been carried out in its core. Since 2000, activities on in-reactor tests of fusion reactor materials have been performed at the WWR-K reactor, such as experiments on tritium release out of lithium ceramics. Tests forced development and fabrication of an installation for in-reactor studies of tritium release from various candidate materials of fusion reactor blankets in the inert gas environment of an ampoule with specimens under study. Also, a technique has been developed for assessment of the time of tritium retention in materials under irradiation.
In 2018, the WWR-K reactor facility was upgraded for studies of fusion reactor materials under irradiation, which makes it possible to carry out experiments on irradiation of specimens at vacuum conditions.
This work presents the experimental facility description and block circuit along with its general technical capacities as applied to the expected studies of tritium release of fusion reactor materials at the WWR-K reactor. The developed irradiation ampoule device is presented schematically as well. Also, the obtained results of the neutron-physical, thermophysical, and vacuum calculations for the in-reactor experiment on irradiation of fusion reactor blanket materials are given.