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Argonne research aims to improve nuclear fuel recycling and metal recovery
Servis
Scientists at Argonne National Laboratory are investigating a used nuclear fuel recycling technology that could lead to a scaled-down and more efficient approach to metal recovery, according to a recent news article from the lab. The research, led by Argonne radiochemist Anna Servis with funding from the Department of Energy’s Advanced Research Projects Agency–Energy (ARPA-E), could have an impact beyond the nuclear fuel cycle and improve other high-value metal processing, such as rare earth recovery, according to Argonne.
The research: Servis’s work is being carried out under ARPA-E’s CURIE (Converting UNF Radioisotopes Into Energy) program. The specific project—Radioisotope Capture Intensification Using Rotating Packed Bed Contactors—started in 2023 and is scheduled to end in January 2026.
S. J. Shin, J. R. I. Lee, T. van Buuren, K. C. Chen, K. A. Moreno, H. Huang, D. E. Hoover, A. Nikroo, A. V. Hamza, S. O. Kucheyev
Fusion Science and Technology | Volume 73 | Number 3 | April 2018 | Pages 467-473
Technical Paper | doi.org/10.1080/15361055.2017.1392181
Articles are hosted by Taylor and Francis Online.
Controlled doping of inertial confinement fusion (ICF) targets is needed to enable nuclear diagnostics of implosions. Here, we demonstrate that ion implantation with a custom-designed carousel holder can be used for azimuthally uniform doping of ICF fuel capsules made from a glow discharge polymer (GDP). Particular emphasis is given to the selection of the initial wall thickness of GDP capsules as well as implantation and postimplantation annealing parameters in order to minimize capsule deformation during a postimplantation thermal treatment step. In contrast to GDP, ion-implanted high-density carbon exhibits excellent thermal stability and ~100% implantation efficiency for the entire range of ion doses studied (2 × 1014 to 1 × 1016 cm−2) and for annealing temperatures up to 700°C. Finally, we demonstrate a successful doping of planar Al targets with isotopes of Kr and Xe to doses of ~1017 cm−2.